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Raquel Portela, Susana Perez-Ferreras, Ana Serrano-Lotina, Miguel A. Bañares
《化学科学与工程前沿(英文)》 2018年 第12卷 第3期 页码 509-536 doi: 10.1007/s11705-018-1740-9
The term operando was coined at the beginning of this century to gather the growing efforts devoted to establish structure-activity relationships by simultaneously characterizing a catalyst performance and the relevant surface chemistry during genuine catalytic operation. This approach is now widespread and consolidated; it has become an increasingly complex but efficient junction where spectroscopy, materials science, catalysis and engineering meet. While for some characterization techniques kinetically relevant reactor cells with good resolution are recently developing, the knowledge gained with magnetic resonance and X-ray and vibrational spectroscopy studies is already huge and the scope of operando methodology with these techniques is recently expanding from studies with small amounts of powdered solids to more industrially relevant catalytic systems. Engineering catalysis implies larger physical domains, and thus all sort of gradients. Space- and time- resolved multi-technique characterization of both the solid and fluid phases involved in heterogeneous catalytic reactions (including temperature data) is key to map processes from different perspectives, which allows taking into account existing heterogeneities at different scales and facing up- and down-scaling for applications ranging from microstructured reactors to industrial-like macroreactors (operating with shaped catalytic bodies and/or in integral regime). This work reviews how operando methodology is evolving toward engineered reaction systems.
关键词: operando structured catalysts space-resolved time-resolved spectroscopy
结构化稀疏学习综述 Review
Lin-bo QIAO, Bo-feng ZHANG, Jin-shu SU, Xi-cheng LU
《信息与电子工程前沿(英文)》 2017年 第18卷 第4期 页码 445-463 doi: 10.1631/FITEE.1601489
关键词: 结构化稀疏学习;算法;应用
《环境科学与工程前沿(英文)》 2023年 第17卷 第6期 doi: 10.1007/s11783-023-1667-3
● Hybrid deep-learning model is proposed for water quality prediction.
关键词: Water quality prediction Soft-sensor Anaerobic process Tree-structured Parzen Estimator
Computational design of structured chemical products
Faheem Mushtaq, Xiang Zhang, Ka Y. Fung, Ka M. Ng
《化学科学与工程前沿(英文)》 2021年 第15卷 第5期 页码 1033-1049 doi: 10.1007/s11705-020-2002-1
关键词: product design performance ingredients structure manufacturing process framework structured chemical products microstructure design
Yali CHEN,Lu XIONG,Weikang WANG,Xing ZHANG,Hanqing YU
《环境科学与工程前沿(英文)》 2015年 第9卷 第5期 页码 897-904 doi: 10.1007/s11783-015-0782-1
关键词: nitrobenzene nano-structured Cu electro-reduction voltage-dependent electrodeposition high selectivity high stability
Property-performance relationship of core-shell structured black TiO photocatalyst for environmental
《环境科学与工程前沿(英文)》 2023年 第17卷 第9期 doi: 10.1007/s11783-023-1711-3
● Properties and performance relationship of CSBT photocatalyst were investigated.
关键词: Black TiO2 Core-shell structure Property-performance relationship Agro-industrial effluent Environmental remediation
Erratum to: Efficient keyword search over graph-structured data based on minimal covered Erratum
Asieh Ghanbarpour, Abbas Niknafs, Hassan Naderi,naderi@iust.ac.ir
《信息与电子工程前沿(英文)》 2020年 第21卷 第6期 页码 809-962 doi: 10.1631/FITEE.18e0133
《能源前沿(英文)》 doi: 10.1007/s11708-023-0898-0
关键词: carbon dioxide electroreduction electrochemistry co-electrodeposition intermetallic catalysts value-added chemicals
《能源前沿(英文)》 doi: 10.1007/s11708-023-0907-3
关键词: oxygen reduction electrocatalysis Pt single-atom catalysts conventional Pt-based catalysts design thoughts and synthesis metal-support interactions
Pengfei JI, Yiming RONG, Yuwen ZHANG, Yong TANG
《能源前沿(英文)》 2018年 第12卷 第1期 页码 137-142 doi: 10.1007/s11708-018-0532-8
关键词: thermoelectric material thermal transport Si/Gesuperlattics molecular dynamics (MD)
Minghou LIU, Yaqing WANG, Dong LIU, Kan XU, Yiliang CHEN
《能源前沿(英文)》 2011年 第5卷 第1期 页码 75-82 doi: 10.1007/s11708-010-0014-0
Promising approach for preparing metallic single-atom catalysts: electrochemical deposition
《能源前沿(英文)》 2022年 第16卷 第4期 页码 537-541 doi: 10.1007/s11708-022-0837-5
Deep convolutional tree-inspired network: a decision-tree-structured neural network for hierarchical
《机械工程前沿(英文)》 2021年 第16卷 第4期 页码 814-828 doi: 10.1007/s11465-021-0650-6
关键词: bearing cross-severity fault diagnosis hierarchical fault diagnosis convolutional neural network decision tree
Current challenge and perspective of PGM-free cathode catalysts for PEM fuel cells
Gang WU
《能源前沿(英文)》 2017年 第11卷 第3期 页码 286-298 doi: 10.1007/s11708-017-0477-3
关键词: oxygen reduction fuel cells cathode nonprecious metal catalysts carbon nanocomposites
Selective preparation for biofuels and high value chemicals based on biochar catalysts
《能源前沿(英文)》 2023年 第17卷 第5期 页码 635-653 doi: 10.1007/s11708-023-0878-4
标题 作者 时间 类型 操作
Water quality soft-sensor prediction in anaerobic process using deep neural network optimized by Tree-structured
期刊论文
Computational design of structured chemical products
Faheem Mushtaq, Xiang Zhang, Ka Y. Fung, Ka M. Ng
期刊论文
Efficient and selective electro-reduction of nitrobenzene by the nano-structured Cu catalyst prepared
Yali CHEN,Lu XIONG,Weikang WANG,Xing ZHANG,Hanqing YU
期刊论文
Property-performance relationship of core-shell structured black TiO photocatalyst for environmental
期刊论文
Erratum to: Efficient keyword search over graph-structured data based on minimal covered
Asieh Ghanbarpour, Abbas Niknafs, Hassan Naderi,naderi@iust.ac.ir
期刊论文
Electrochemical CO reduction to C products over CuZn intermetallic catalysts synthesized by electrodeposition
期刊论文
Oxygen reduction electrocatalysis: From conventional to single-atomic platinum-based catalysts for proton
期刊论文
Impacts of cone-structured interface and aperiodicity on nanoscale thermal transport in Si/Ge superlattices
Pengfei JI, Yiming RONG, Yuwen ZHANG, Yong TANG
期刊论文
Experimental study of the effects of structured surface geometry on water spray cooling performance in
Minghou LIU, Yaqing WANG, Dong LIU, Kan XU, Yiliang CHEN
期刊论文
Deep convolutional tree-inspired network: a decision-tree-structured neural network for hierarchical
期刊论文